Erickson ML, Yager RM, Kauffman LJ, Wilson JT. Drinking water quality in the glacial aquifer system, northern USA. Sci Total Environ. 2019 Aug 2;694:133735. doi: 10.1016/j.scitotenv.2019.133735
Groundwater supplies 50% of drinking water worldwide, but compromised water quality from anthropogenic and geogenic contaminants can limit usage of groundwater as a drinking water source. Groundwater quality in the glacial aquifer system, USA (GLAC), is presented in the context of a hydrogeologic framework that divides the study area into 17 hydrogeologic terranes. Results are reported at aquifer-system scale and regional (terrane) scale. This paper presents a quantitative assessment of groundwater quality in the GLAC using data from numerous sources for samples collected 2005-2013, compared to health-based and aesthetic (non-health) benchmarks, and evaluated with areal and population metrics. Concentrations above a benchmark are considered high. Trace elements are widespread across the study area, with an estimated 5.7 million people relying on groundwater with high concentrations of one or more trace elements; manganese and arsenic are most often at high concentration. Nitrate is found at high concentration in 4.0% of the study area, serving about 740 thousand people. Organic compounds including pesticides and volatile organic compounds are high in 2.0% of the assessed study area, with about 870 thousand people relying on groundwater with high concentrations of an organic compound. High arsenic and manganese concentrations occur primarily in the terranes with thick, stratigraphically complex, fine-grained glacial sediment, coincident with groundwater under reducing conditions (indicated by iron concentrations >100 μg/L); high nitrate is uncommon in those same terranes. When nitrate is high in thick, fine-grained, complex terranes, though, it is much more commonly associated with groundwater under more oxidizing conditions. Common geogenic trace elements occur at high concentration due to characteristic geologic and geochemical conditions. Conversely, anthropogenic nitrate and organic compounds are introduced at or near the land surface. High concentrations of nitrate or organic compounds are generally limited to areas in proximity where people live and use the chemicals.
Thamires de Oliveira Moura, Franciele, Palmeira Campos, Iara Brandão, Yvonilde Dantas Pinto Medeiros. Inorganic and organic contaminants in drinking water stored in polyethylene cisterns Food Chemistry, Volume 273, 1 February 2019. https://doi.org/10.1016/j.foodchem.2018.03.104
This work evaluated the presence of contaminants in stored rainwater in 36 polyethylene tanks installed in two rural communities of the semiarid of Bahia, Brazil. Carbonyl compounds were analyzed by High Performance Liquid Chromatography (HPLC-UV), BTEX (Benzene, Toluene, Ethylbenzene and Xylenes) by gas chromatoghaphy (GC-FID), and trace elements by inductively coupled plasma optical emission spectrometry (ICP-OES). Seven carbonyl compounds were quantified including acrolein (<3–115 µg L−1), which is considered a potent mutagenic agent, above the potability limit in 75% of the cases. Trace elements such as copper, zinc, barium, aluminum and lead, more frequently found, were also quantified, and lead (<0,56–99 µg L−1) was above the tolerable limit for drinking water of 10 μg L−1 in 73% of the cases. The results show that the stored water in polyethylene cisterns in the Brazilian semiarid region does not present satisfactory conditions for human consumption.
Di M, Liu X, Wang W, Wang J. Manuscript prepared for submission to environmental toxicology and pharmacology pollution in drinking water source areas: Microplastics in the Danjiangkou Reservoir, China. Environmental toxicology and pharmacology. 2018 Dec 17;65:82-89. doi: 10.1016/j.etap.2018.12.009.
As the source of water for the South-to-North Water Diversion Project of China, the water quality of the Danjiangkou Reservoir (DJKR) is related to the safety of drinking water for billions of residents. Consequently, microplastics in surface water and sediment samples of the DJKR were investigated in this study. Microplastics were observed in all water and sediment samples with abundances varying from 467 to 15,017 n/m3 and 15 to 40 n/kg wet weight, respectively. Microplastics were rich in colour and dominated by fibrous items. Small-sized particles (< 2 mm) were more frequently observed than other sizes. Analysis by micro-Raman spectroscopy showed that polypropylene was the major polymer type. These systematic results demonstrated that the DJKR is suffering from the pollution of microplastics, which should be paid more attention based on its potential threat to the aquatic organisms and residents impacted by the drinking water source pollution.
Qu B, Zhang Y, Kang S, Sillanpää M. Water quality in the Tibetan Plateau: Major ions and trace elements in rivers of the “Water Tower of Asia”. Sci Total Environ. 2018 Aug 25;649:571-581. doi: 10.1016/j.scitotenv.2018.08.316.
As the “Water Tower of Asia”, rivers originating from the Tibetan Plateau provide water resources for more than one billion residents in both its local and surrounding areas. With respect to the essential role that this region plays in terms of water resources in Asia, we provide an overview of the mechanisms governing the water quality, including the major ions and trace elements release, in eleven rivers of the Tibetan Plateau. Overall, the rivers running on the Tibetan Plateau reflect an alkaline aquatic environment, with an average pH of 8.5; and the total dissolved solids (TDS, ~339 mg L-1) are much higher than the global average value. Over 80% of the water ionic budget in the rivers of the plateau is comprised of Ca2+, Mg2+, HCO3- and SO42-. The main mechanisms that control the river water chemistry on the Tibetan Plateau are natural processes and present a visible spatial heterogeneity. For instance, in rivers of the southern Tibetan Plateau, the water quality is mainly controlled by the rock-weathering, while rivers of the central and northern Tibetan Plateau are also largely affected by evaporation-crystallization processes. In general, most of the rivers on the Tibetan Plateau are uncontaminated and still in a pristine condition. However, it should be noted that due to the natural process such as rock-weathering and groundwater leaching, and anthropogenic activities such as urbanization and mining operations, the concentrations of several toxic elements (e.g., As, Cd, Pb, Mn, Hg and Tl) in some of the basins are higher than the China national standard (GB) and the World Health Organization (WHO) guidelines for drinking water. With increasing anthropogenic activities on the plateau and changes in the river basins, it is necessary to conduct the long-term monitoring of the river water chemistry of this climate-sensitive and eco-fragile region.
Islam MMM, Iqbal MS, Leemans R, Hofstra N. Modelling the impact of future socio-economic and climate change scenarios on river microbial water quality. International journal of hygiene and environmental health. 2017 Dec 4. pii: S1438-4639(17)30408-X. doi: 10.1016/j.ijheh.2017.11.006.
Microbial surface water quality is important, as it is related to health risk when the population is exposed through drinking, recreation or consumption of irrigated vegetables. The microbial surface water quality is expected to change with socio-economic development and climate change. This study explores the combined impacts of future socio-economic and climate change scenarios on microbial water quality using a coupled hydrodynamic and water quality model (MIKE21FM-ECOLab). The model was applied to simulate the baseline (2014-2015) and future (2040s and 2090s) faecal indicator bacteria (FIB: E. coli and enterococci) concentrations in the Betna river in Bangladesh. The scenarios comprise changes in socio-economic variables (e.g. population, urbanization, land use, sanitation and sewage treatment) and climate variables (temperature, precipitation and sea-level rise). Scenarios have been developed building on the most recent Shared Socio-economic Pathways: SSP1 and SSP3 and Representative Concentration Pathways: RCP4.5 and RCP8.5 in a matrix. An uncontrolled future results in a deterioration of the microbial water quality (+75% by the 2090s) due to socio-economic changes, such as higher population growth, and changes in rainfall patterns. However, microbial water quality improves under a sustainable scenario with improved sewage treatment (-98% by the 2090s). Contaminant loads were more influenced by changes in socio-economic factors than by climatic change. To our knowledge, this is the first study that combines climate change and socio-economic development scenarios to simulate the future microbial water quality of a river. This approach can also be used to assess future consequences for health risks.
Li F, Qiu Z, Zhang J, Liu C, Cai Y, Xiao M. Spatial Distribution and Fuzzy Health Risk Assessment of Trace Elements in Surface Water from Honghu Lake. International journal of environmental research and public health. 2017 Sep 4;14(9). pii: E1011. doi: 10.3390/ijerph14091011.
Previous studies revealed that Honghu Lake was polluted by trace elements due to anthropogenic activities. This study investigated the spatial distribution of trace elements in Honghu Lake, and identified the major pollutants and control areas based on the fuzzy health risk assessment at screening level. The mean total content of trace elements in surface water decreased in the order of Zn (18.04 μg/L) > Pb (3.42 μg/L) > Cu (3.09 μg/L) > Cr (1.63 μg/L) > As (0.99 μg/L) > Cd (0.14 μg/L), within limits of Drinking Water Guidelines. The results of fuzzy health risk assessment indicated that there was no obvious non-carcinogenic risk to human health, while carcinogenic risk was observed in descending order of As > Cr > Cd > Pb. As was regarded to have the highest carcinogenic risk among selected trace elements because it generally accounted for 64% of integrated carcinogenic risk. Potential carcinogenic risk of trace elements in each sampling site was approximately at medium risk level (10-5 to 10-4). The areas in the south (S4, S13, and S16) and northeast (S8, S18, and S19) of Honghu Lake were regarded as the risk priority control areas. However, the corresponding maximum memberships of integrated carcinogenic risk in S1, S3, S10-S13, S15, and S18 were of relatively low credibility (50-60%), and may mislead the decision-makers in identifying the risk priority areas. Results of fuzzy assessment presented the subordinate grade and corresponding reliability of risk, and provided more full-scale results for decision-makers, which made up for the deficiency of certainty assessment to a certain extent.
Zhang HW, Sun YQ, Li Y, Zhou XD, Tang XZ, Yi P, Murad A, Hussein S, Alshamsi D, Aldahan A, Yu ZB, Chen XG, Mugwaneza VDP. Quality assessment of groundwater from the south-eastern Arabian Peninsula. Environ Monit Assess. 2017 Aug;189(8):411. doi: 10.1007/s10661-017-6092-2.
Assessment of groundwater quality plays a significant role in the utilization of the scarce water resources globally and especially in arid regions. The increasing abstraction together with man-made contamination and seawater intrusion have strongly affected groundwater quality in the Arabia Peninsula, exemplified by the investigation given here from the United Arab Emirates, where the groundwater is seldom reviewed and assessed. In the aim of assessing current groundwater quality, we here present a comparison of chemical data linked to aquifers types. The results reveal that most of the investigated groundwater is not suitable for drinking, household, and agricultural purposes following the WHO permissible limits. Aquifer composition and climate have vital control on the water quality, with the carbonate aquifers contain the least potable water compared to the ophiolites and Quaternary clastics. Seawater intrusion along coastal regions has deteriorated the water quality and the phenomenon may become more intensive with future warming climate and rising sea level.